Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Yokoyama, Tatsunori
Isotope News, (764), p.11 - 14, 2019/08
no abstracts in English
Matsushima, Ryotatsu; Sato, Fuminori; Saito, Yasuo; Atarashi, Daiki*
Proceedings of 3rd International Symposium on Cement-based Materials for Nuclear Wastes (NUWCEM 2018) (USB Flash Drive), 4 Pages, 2018/10
At TRP, LWTF was constructed as a facility for processing low radioactive liquid waste and solid waste generated at TRP, and a cold test is been carrying out. In this facility, initially, nitrate waste liquid after separation of nuclides generated with treatment of low radioactive liquid waste was to be solidified by using borate. However, at present, it is necessary to decompose the nitrate in the liquid waste to reduce the environmental burden. For the reason, as a plan to replace the nitrate with the carbonate and to make it as a cement based encapsulation, we are studying for the introduction of the facility. Currently, as a cement solidification technology development for this liquid waste, we are studying the application of cement material based on blast furnace slag (BFS) as a main component. In this report, we show the results of the test conducted on the actual scale (200 L drum can scale).
Horiike, Takumi*; Dotsuta, Yuma*; Nakano, Yuriko*; Ochiai, Asumi*; Utsunomiya, Satoshi*; Onuki, Toshihiko; Yamashita, Mitsuo*
Applied and Environmental Microbiology, 83(20), p.e00855-17_1 - e00855-17_11, 2017/10
Times Cited Count:18 Percentile:62.48(Biotechnology & Applied Microbiology)Radioactive strontium (Sr) leaked into the ocean from the Fukushima Daiichi Nuclear Power Plant after the nuclear accident. Since the removal of Sr using general adsorbents is not efficient at high salinity, this study investigated removal of soluble Sr from a saline solution by biogenic carbonate minerals. An isolate, Bacillus sp. strain TK2d, from marine sediment removed more than 99 % of Sr in a saline solution. Sr adsorbed at the cell surface and then carbonate minerals containing Sr developed outside the cells.
Nagaishi, Ryuji; Motooka, Takafumi; Yamagishi, Isao
Proceedings of 2016 EFCOG Nuclear & Facility Safety Workshop (Internet), 6 Pages, 2016/09
Overflow of water from waste storage tanks of High Integrity Containers (HIC) in the multi-nuclide removal equipment (ALPS) was discovered at Fukushima Daiichi NPS in April of last year. The mechanism of overflow was not understood very much at that time. To elucidate that for chemical safety in the waste storage, irradiation experiments of simulated carbonate slurry by Co-60 -rays have been conducted in CLADS, JAEA in cooperation with TEPCO, TOSHIBA and KURITA. Hydrogen molecule was the main radiolytic gas product in the slurry, and its amount was enhanced by dissolved species of not only halide ions as seawater components but also carbonate ion as an additive for co-precipitation at a basic condition. The bubbles of molecules were further formed and almost held in the slurry without stirred. These sequentially led to the expansion of slurry, and then to its separation into the shrunk one and supernatant water, which was little accumulated without irradiated.
Iida, Yoshihisa; Barr, L.; Yamaguchi, Tetsuji; Hemmi, Ko
Genshiryoku Bakkuendo Kenkyu (CD-ROM), 23(1), p.3 - 8, 2016/06
Thorium (Th)-229 is one of the important radionuclides for the performance assessment calculations for high-level radioactive waste repositories. The sorption behavior of Th onto montmorillonite and illite were investigated by batch sorption experiments. Experiments were carried out under variable pH and carbonate concentrations. The sorbability of montmorillonite was higher than that of illite. Distribution coefficients, (m kg), decreased with increased carbonate concentrations and showed the minimal value at around pH 10. The sorption behaviors of Th were analyzed by the non-electrostatic surface complex model with PHREEQC computer program. The model calculations were able to explain the experimental results reasonably well. The decreases of was likely due to the stabilization of aqueous species by hydroxo-carbonate complexations in the solutions.
Yamaguchi, Tetsuji; Nakayama, Shinichi
JAERI-Conf 2003-018, p.115 - 116, 2003/10
Effective diffusivity was determined for Np(IV) in bentonite material in presence of carbonate and for Pu(IV) in presence of fulvic acid. Adsorption of actinides onto negatively charged mineral surfaces were investigated under conditions that actinides were predominantly present as anionic complex species. The results of this study will reveal behavior of actinides under various geological environments.
Nagaishi, Ryuji; Kimura, Takaumi; Sinha, S. P.*
Molecular Physics, 101(7), p.1007 - 1014, 2003/01
Times Cited Count:20 Percentile:52.7(Chemistry, Physical)no abstracts in English
Yamaguchi, Tetsuji; Nakayama, Shinichi; Okamoto, Hisato
Radiochimica Acta, 90(12), p.863 - 868, 2003/01
Times Cited Count:4 Percentile:29.2(Chemistry, Inorganic & Nuclear)no abstracts in English
Lee, S.; Kondoh, Takashi; Miura, Yukitoshi
Japanese Journal of Applied Physics, Part 1, 41(11A), p.6574 - 6576, 2002/11
Times Cited Count:1 Percentile:5.59(Physics, Applied)no abstracts in English
Chiba, Shinichi; Kawano, Yasunori; Tsuchiya, Katsuhiko; Inoue, Akira*
JAERI-Research 2001-050, 59 Pages, 2001/11
no abstracts in English
Lee, S.; Kondoh, Takashi; Miura, Yukitoshi
Purazuma, Kaku Yugo Gakkai-Shi, 77(9), p.919 - 929, 2001/09
no abstracts in English
Yamaguchi, Tetsuji
Kyouto Daigaku Daigakuin Kougaku Kenkyuka Hakase Gakui Ronbun, 136 Pages, 2001/01
no abstracts in English
JNC TN8400 2000-030, 17 Pages, 2000/12
As a representative of natural marine groundwater, the author selected pumped water from a Quaternary sedimentary aquifer of the Mobara gas-field in Japan and measured the concentration of total organic carbon (TOC) and of organic acid anions (formic, acetic, lactic, succinic, humic, fulvic, propionic, valeric and butyric acids). The concentration of TOC ranged from 221 to 240mg/L. As organic acid anions, only succinic and fulvic acids were detected and each concentration was given to be from 5.8 0.5 to 8.30.3 and from 3.30.2 to 3.50.2mg/L, respectively. By consideration of the temperature and the [SO] of the groundwater, it is inferred that the organic acid has been significantly decomposed by activities of microbes, such as the fermentation process, CHCOO + HO = HCO + CH.
Lee, S.; Kondoh, Takashi; Yonemoto, Y.*; Miura, Yukitoshi
Review of Scientific Instruments, 71(12), p.4445 - 4448, 2000/12
Times Cited Count:6 Percentile:44.13(Instruments & Instrumentation)no abstracts in English
; ; *; Yamaguchi, Akira
JNC TN9400 2000-109, 96 Pages, 2000/11
Numerical calculations were carried out for a free surface sloshing, a thermal stratification, a thermal striping, and a natural convection as key phenomena of in-vessel thermohydraulics in future fast reactor systems with various fluids as coolants. This numerical work was initiaied based on a recognition that the fundamental characteristics of the phenomena have been unsolved quantitatively in the use of various coolants. From the analysis for the phenomena, the following results were obtained. [Free Surface Sloshing phenomena] (1)Ther is no remarkable difference betweeen liquid sodium and luquid Pb-Bi in characteristics of internal flows and free surface charatristics based on Fr number. (2)the AQUA-VOF code has a potentiall enough to evaluate gas entrainment behavior from the free surface including the internal flow characteristics. [thermal Stratification Phenomena] (1)On-set position of thermal entainment process due to dynamic vortex flows was moved to downstream direction with decreasing of Ri number. 0n the other hand, the position in the case of C0 gas was shifted to upstream side with decreasing of Ri number. (2)Destruction speed of the thermal stratyification interface was dependent on thermal diffusivity as fluid properties. therefor it was concluded that an elimination method is necessary for the interface generated in C0 gas. [thermal Striping Phenomena] (1)Large amplitudes of fluid temperature fluctuations was reached to down stream area in the use of CO gas, due to larger fluid viscosity and smaller thermal diffusivity, compared with liquid sodium and liquid Pb-Bi cases. (2)To simulate thermal striping conditions such as amplitude and frequency of the fluid temperature fluctuations, it isnecessary for coincidences of Re number for the amplitude and of velocity value for the frequency, in various coolants. [Natural Convection Phenomena] (1)Fundamental behavior of the natural convection in various coolant follows buoyant jet ....
Lee, S.; Kondoh, Takashi
Review of Scientific Instruments, 71(10), p.3718 - 3722, 2000/10
Times Cited Count:4 Percentile:36.73(Instruments & Instrumentation)no abstracts in English
; Yamaguchi, Akira
JNC TN9400 2000-056, 150 Pages, 2000/05
[Purpose] The work was performed to make clear thermal-hydraulic issues resulting in the use of various coolants for fast reactors. [Method] Plant design features due to a use of working fluid other than sodium and design concepts relating a simplification of safety related systems were investigated. And based on the results, quantitative evaluation was made on the topical themal-hydraulic issues. Then both thermal stratification and striping phenomena were evaluated by the used of thermo-hydraulics computer programs. [Results] (1)Thermal-hydraulic issues Topical thermal-hydraulic issues of gaseous and heavy metal cooled reactors were extracted. (a)Gas cooled reactors : natural circulation,flow-induced vibration, depressurization accident (b)Heavy metal cooled reactors : thermal stratification, flow-induced vibration, sloshing And also the thermal-hydraulic issues relating compact reactor assembly and RVACS were extracted resulting from a simplification of safety related systems. (2)Evaluation of thermal stratification and striping phenomena. The following order of affects for the phenomena was obtained: (a) Thermal stratification: CO Sodium Lead, (b) Thermal Striping: CO Lead Sodium
; ; Mizuta, Shunji
JNC TN9400 2000-040, 41 Pages, 2000/03
The corrosion behavior of ferritic stainless steels applied to core components under C0 gas environment was investigated in order to be helpful to fuel design in C0 gas cooled reactor as the feasibility study for fast breeder reactor. The dependence of the corrosion behavior, before a breakaway occurs, on C0 gas temperature, Si and Cr contents of ferritic steels was determined quantitatively. The following correlations to calculate the metal loss thickness was established. X = 4.4w w = √(kt) k = exp( - 5.45[Si]) exp( - 1.09[Cr]) exp( - 11253/T) = 1.65 104.40 10 X : metal loss thickness[ml, w : corrosion weight gain [mg/cm] k : parabola constant [(mg/cm)/hr], t : time [hr], : constant [Si] : Si content[wt.%], [Cr] : Cr content [wt.%], T : temperature [K]
Mizuta, Shunji; ;
JNC TN9400 2000-032, 38 Pages, 2000/03
lt is necessary for feasibility study of fast reactor to evaluate the oxidation of the austenitic stainless steels in the case of using for core material in carbon dioxide gas-cooled reactor. The properties for oxidation of austenitic stainless steels in carbon dioxide were surveyed in literatures and the data were selected after evaluation of factors for oxidation in carbon dioxide. The equation of oxidation in carbon dioxide for PE16, 20Cr/25Ni/Nb, 18Cr-8Ni and JNC Cladding materials were proposed. The equation for oxidation of austenitic stainless steels were expressed as upper limit for the equation according to parabolic law. The equation for JNC cladding materials (PNC316, PNC1520, 14Cr-25Ni) was proposed based the oxidation behavior of 18Cr-8Ni which is same oxidation region for weight gain in three-component system of Fe-Cr-Ni, in addition to evaluate of effect for silicon content. The oxidation equation of 20Cr/25Ni/Nb was applied to the high Ni alloy of JNC cladding material. The obtained equation is as follows, X = 4.4W1000, W = , kp = exp(-Q/(RT)), X: oxide thickness[m], W : weight gain[gcm], kp : parabolic rate constant[gcm s], t :time[sec] : constant[gcmS], Q : activation energy[J・mol], R : gas constant[8.314J K mol], T : temperature[K] (1) PE16 : kp = 1.09010 exp(-192,500/(RD)), (2) 20Cr/25Ni/Nb : kp = 1.65110 exp(-201,300/(RT)) High Ni alloy (JNC), (3)18Cr-8Ni : kp = 1.50310 exp(-60,000/(RT)), (4) PNC316, PNC1520 : kp = 1.50310 exp(-60,000/(RT))0.62 14Cr-25Ni(JNC) The weight gain is (3)(4)(2)(1) in order.